Bui Van Loat, Le Tuan Anh, Nguyen Van Quan, Dinh Van Thin, Nguyen Cong Tam

Main Article Content

Abstract

Abstract. In this work the non-destructive gamma - spectroscopic method for determination of uranium enrichment is presented. The method is applicable to material of any physical form and geometrical shape, and does not require the use of reference materials or the use of efficiency calibrated geometry. The X Rays and gamma rays below 100 keVfrom 235U were used to determine their relative detection efficiency internally. The activity ratios of 234U/235U and U238/U235in studied sample were calculated based on the measurents of the count rate of 53.2keV (0.123%) gamma ray of 234U and 92.6 keV (5.16%) of 234Th, a daughter of 238U.  As a test of this method, a highly enriched uraniumsample was measured. The obtained result was in agreement with the estimated value.

Keywords: Uranium enrichment, gamma-spectrometry, intrinsic efficiency calibration, MGA method.

References

[1] A Luca, Experimental Determination of the Uranium Enrichment Ratio, Rom.Journ.Phys,Vol 53, Nos. 1- 2,P35 -39, Bucharest,2008.
[2] Y.Y. Ebaid, Use of gamma-ray spectrometry for uranium isotopic analysis in environmental samples, Rom. Journ. Phys. Vol.55,Nos 1-2 P69-74, Bucharest,2010.
[3] H. Yucel, H.Dikmen, Uranium enrichment measurements using the intensity ratios of self- fluresence X- ray-92*keV gamma ray in UXKα spectral region, Talanta 78 (2009) pp 410-417.
[4] W.D. Ruhter et all, Uranium enrichment measurement without calibration using gamma ray above 100 KeV, Sym.on International Safeguards; Verification and Nuclear Material Security Vienna,Austra; October 29- November 1,2001,p1-4.
[5] L.T.Anh, N.C.Tam, B.V.Loat- Determination some parameter of uranium material by gamma spectrometry using intrinsic eficiency calibration- Proceeding of the topical conference on nuclear physics, hihg energy physics and astrophysics ( NPHEAP-2010) 283-288.
[6] C.T. Nguyen, J. Zsigrai, Gamma-spectrometric uranium age-dating using intrisic efficiency calibration, Nucl. Instr. And Meth. B 243 (2006) 187.
[7] M.H. Nassef, W.EI Monwafi, and M.S.EI Tahawy. Non desteuctive assay for 235U determination in reference materials of uranium oxide. Journal of Nuclear and Radiation Physics. Vol 4, No2,2009,pp65-73.
[8] D.J. Karangelosanf et all, Determination of depleted uranium in environmental samples by gamma- spectroscopic techniques. Jour. of EnvironnmentalRadioactivity 76 (2004) 294-310
[9] HalukYÜcel, The applicability of MGA method for depleted and natural uranium isotopic analysis in the presence of actinides, Applied Radiation and Isotopies 65 (2007) 1269-1280.
[10] Delynn Clark, U235 A gamma ray analysis code for uranium isotopic determination, Lawrence Livermore National Laboratory, 1996